Reversible reaction and diffusion within a porous catalyst slab

A. L. Paiva, F. X. Malcata*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

9 Citations (Scopus)

Abstract

This study elucidates how integration of reaction and separation can bring about enhancement of effectiveness factors via consideration of a catalyst immobolized onto a porous slab-shaped bead which catalyzes a reversible reaction where the reactant and the product possess different apparent diffusivities. The porous support is assumed to play the dual role of avoiding loss of the catalyst in the reactor/separator effluent stream and bring about in situ separation of reactant and product. In order to simplify the model situation and allow analytical reasoning to be followed throughout, only reversible first-order kinetics in an ideal binary system are considered.

Original languageEnglish
Pages (from-to)4429-4432
Number of pages4
JournalChemical Engineering Science
Volume52
Issue number23
DOIs
Publication statusPublished - Dec 1997

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